High-Performance Vanadium Redox Flow Battery with Polyacrylic Acid-Bound Carbon Nanoparticles on Graphite Felts

Document Type

Article

Source of Publication

Journal of the Electrochemical Society

Publication Date

3-1-2025

Abstract

Power density enhancement is crucial for cost reduction and increased commercial viability of vanadium redox flow batteries (VRFB). The low performance of commercially used porous graphite felt electrodes is the main limiting factor in increasing the power density of such devices. Herein, we introduce a novel approach to improve electrode activity and conductivity by loading a considerable amount of carbon black nanoparticles on the graphite fibers using polyacrylic acid as a primary mucoadhesive polymer. The prepared electrode structure showed prominent inter-fiber connections, as evidenced by scanning electron microscope images, which significantly reduced the ohmic resistance and improved electron transfer. Galvanostatic charge-discharge profiles showed 12%-15% higher energy efficiencies at current densities ranging from 50 to 150 mA cm−2 compared to thermally treaded felts with no signs of degradation after fifty cycles, marking a promising advancement in VRFB technology.

ISSN

0013-4651

Publisher

The Electrochemical Society

Volume

172

Issue

3

Disciplines

Engineering

Keywords

carbon black, electrode, graphite felt, poly acrylic acid, vanadium redox flow batteries

Scopus ID

05002029349

Indexed in Scopus

yes

Open Access

no

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